Raman spectroscopy of infrared multiphoton excited molecules

Presentation Date: 

Wednesday, January 1, 1986

Location: 

XIVth Int. Quantum Electronics Conf. (San Francisco, CA)
Anti-Stokes signals from various modes of isolated, infrared multiphoton excited SF6 and C2H4F2 molecules are measured as a function of pressure, infrared fluence and wavelength. This allows to verify whether intramolecular equilibrium of vibrational energy is established after infrared multiphoton excitation in isolated molecules.